An Overview of Coacervates: The Special Disperse State of Amphiphilic and Polymeric Materials in Solution

⚡ 摘要

凝聚层综述:两亲性和高分子材料在溶液中的特殊分散状态

作者 Satya P. Moulik; Animesh Kumar Rakshit; Animesh Pan; Bappaditya Naskar 期刊 Colloids and Interfaces 发表日期 2022 ISSN 2504-5377 DOI 10.3390/colloids6030045 类型 原创研究 (Original Research)

📄 英文摘要 English Abstract

EN

Individual amphiphiles, polymers, and colloidal dispersions influenced by temperature, pH, and environmental conditions or interactions between their oppositely charged pairs in solvent medium often produce solvent-rich and solvent-poor phases in the system. The solvent-poor denser phase found either on the top or the bottom of the system is called coacervate. Coacervates have immense applications in various technological fields. This review comprises a concise introduction, focusing on the types of coacervates, and the influence of different factors in their formation, structures, and stability. In addition, their physicochemical properties, thermodynamics of formation, and uses and multifarious applications are also concisely presented and discussed.

📄 中文摘要 Chinese Abstract

中文
在溶剂介质中,受温度、pH值、环境条件影响或相反电荷对之间相互作用的单个两亲分子、聚合物和胶体分散体系,往往会在体系中产生富溶剂相和贫溶剂相。体系中位于顶部或底部的贫溶剂致密相被称为凝聚层。凝聚层在各类技术领域具有广泛的应用价值。

📋 英文结构化总结 English Structured Summary

全文整理

EN

Background:

Individual amphiphiles, polymers, and colloidal dispersions influenced by temperature, pH, and environmental conditions or interactions between their oppositely charged pairs in solvent medium often produce solvent-rich and solvent-poor phases in the system. The solvent-poor denser phase found either on the top or the bottom of the system is called coacervate. Coacervates have immense applications in various technological fields.

Methods:

N/A - Review article

Results:

This review comprises a concise introduction, focusing on the types of coacervates, and the influence of different factors in their formation, structures, and stability. In addition, their physicochemical properties, thermodynamics of formation, and uses and multifarious applications are also concisely presented and discussed. The review covers theories of coacervation, methods used for the determination of coacervates properties, and factors influencing coacervation including ionic strength, pH, molecular weight, chirality, charge density, temperature, and solvent. It also details coacervate types (simple and complex, including polyelectrolyte–polyelectrolyte, polyelectrolyte–surfactant, surfactant–surfactant, and peptide/protein types), their preparation, and properties.

Data Summary:

The review systematically categorizes coacervate types and the specific factors influencing their formation, such as ionic strength, pH, molecular weight, chirality, charge density, temperature, and solvent. It also outlines distinct application areas for coacervates, including wastewater treatment, protein purification, food formulation, cellular mimics, nanoparticle synthesis, and delivery carriers.

Conclusions:

Coacervates represent a special disperse state of amphiphilic and polymeric materials in solution, formed as a solvent-poor denser phase under various environmental conditions or through interactions of oppositely charged pairs. Their formation, structures, stability, physicochemical properties, and thermodynamics are significantly influenced by multiple system parameters.

Practical Significance:

Coacervates possess immense applications in various technological fields, serving practical roles in wastewater treatment, protein purification, food formulation, cellular mimics, nanoparticle synthesis, and as delivery carriers.

📋 中文结构化总结 Chinese Structured Summary

中文

背景:

在溶剂介质中,受温度、pH值、环境条件影响或相反电荷对之间相互作用的单个两亲分子、聚合物和胶体分散体系,往往会在体系中产生富溶剂相和贫溶剂相。体系中位于顶部或底部的贫溶剂致密相被称为凝聚层。凝聚层在各类技术领域具有广泛的应用价值。

方法:

不适用——综述类文章

结果:

本综述包括一个简明的引言,重点介绍凝聚层的类型以及不同因素对其形成、结构和稳定性的影响。此外,还简明地介绍和讨论了其物理化学性质、形成热力学及其用途和多种应用。综述涵盖了凝聚理论、用于测定凝聚层性质的方法,以及影响凝聚的因素,包括离子强度、pH值、分子量、手性、电荷密度、温度和溶剂。同时详细阐述了凝聚层的类型(简单凝聚层和复杂凝聚层,包括聚电解质-聚电解质型、聚电解质-表面活性剂型、表面活性剂-表面活性剂型以及肽/蛋白质型)、其制备方法及性质。

数据总结:

本综述系统地将凝聚层类型及其形成的具体影响因素进行了分类,包括离子强度、pH值、分子量、手性、电荷密度、温度和溶剂。同时概述了凝聚层的不同应用领域,包括废水处理、蛋白质纯化、食品配方、细胞模拟物、纳米颗粒合成以及作为递送载体。

结论:

凝聚层代表了溶液中的两亲性材料和聚合物材料的一种特殊分散状态,是在各种环境条件下或通过相反电荷对之间的相互作用形成的贫溶剂致密相。其形成、结构、稳定性、物理化学性质和热力学受多种体系参数的显著影响。

实际意义:

凝聚层在各类技术领域具有广泛的应用价值,在废水处理、蛋白质纯化、食品配方、细胞模拟物、纳米颗粒合成以及作为递送载体等方面发挥着实际作用。

📖 中文全文 Chinese Full Text

中文

# 胶体与界面

## 综述

## 凝聚体概述:溶液中两亲性和聚合物材料的特殊分散状态

Satya Priya Moulik¹, Animesh Kumar Rakshit², Animesh Pan³,* 和 Bappaditya Naskar⁴,*

¹ 表面科学中心,贾达夫普尔大学化学系,加尔各答 700032,印度 ² 印度表面科学与技术学会,贾达夫普尔大学化学系,加尔各答 700032,印度 ³ 化学工程系,罗德岛州大学,南金斯敦,RI 02881,美国 ⁴ 化学系,孙德尔本斯·哈齐·德萨拉特学院,加尔各答大学,帕坦卡利 743611,印度

* 通讯作者:animeshpan555@gmail.com (A.P.); bappadityanaskar25@yahoo.com (B.N.)

**摘要:** 受温度、pH值和环境条件影响,或在溶剂介质中带相反电荷的组分之间发生相互作用时,单个两亲分子、聚合物和胶体分散体系往往会在体系中产生富溶剂相和贫溶剂相。体系中位于顶部或底部的贫溶剂致密相称为凝聚体(coacervate)。凝聚体在各类技术领域具有广泛的应用。本综述简要介绍了凝聚体的类型,以及不同因素对其形成、结构和稳定性的影响。此外,还简要介绍和讨论了凝聚体的物理化学性质、形成热力学及其多种多样的应用。

**关键词:** 聚电解质;聚合物;表面活性剂;蛋白质;肽;凝聚体;应用

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**目录**

- 摘要 - 1. 研究背景与展望 - 2. 凝聚理论 - 3. 凝聚体性质测定方法 - 4. 影响凝聚的因素 - 4.1 离子强度 - 4.2 pH值 - 4.3 分子量 - 4.4 手性 - 4.5 电荷密度 - 4.6 温度 - 4.7 溶剂 - 5. 凝聚体的类型、制备与性质 - 5.1 简单凝聚体 - 5.2 复合凝聚体 - 5.2.1 聚电解质-聚电解质型 - 5.2.2 聚电解质-表面活性剂型 - 5.2.3 表面活性剂-表面活性剂型 - 5.2.4 肽/蛋白质型 - 6. 凝聚体的应用 - 6.1 废水处理 - 6.2 蛋白质纯化 - 6.3 食品配方 - 6.4 细胞模拟 - 6.5 纳米颗粒合成 - 6.6 递送载体 - 7. 总结